To improve the conductivity of recently reported single-ionic lithium orthoaluminate complex polymer electrolytes, the structure of the complex unit was changed from [Al(OR) 4 ] - to [Al(SR) 4 ] -, carrying a larger anion radius. The ionic conductivity of such thioaluminate polymer complexes was about 10 - 5 S cm - 1 at room temperature, which was about 10 2 times higher than that of previously reported aluminate complexes. The single-ionic nature of thioaluminate polymer complexes was confirmed by transport number.
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Onishi et al. (1998) studied this question.
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