Hartree-Fock equations are derived for an inert gas adsorbed on a solid surface for the case of highly mobile physisorption. The temperature and pressure dependence of the coverage is calculated and an effective coverage-dependent surface potential is derived. Single-particle energies and wave functions for adsorbed particles are computed yielding the coverage dependence of the adsorbate density profile and adlayer separations. Gas-solid systems studied numerically are ³He on graphite, ⁴He on graphite, and Ar on silver.
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Summerside et al. (1982) studied this question.
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