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January 1, 2017Energy & Environmental ScienceOpen Access

Material design of high-capacity Li-rich layered-oxide electrodes: Li 2 MnO 3 and beyond

Soo Kim Muratahan Aykol Vinay I. Hegde Zhi Lu Scott Kirklin Jason R. Croy Michael M. Thackeray Chris Wolverton

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Abstract

Material design of new Li-rich Li 2 (M I ,M II )O 3 layered oxides for high-energy-density lithium-ion batteries via multi-faceted high-throughput density function theory calculations.

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Kim et al. (2017) studied this question.

synapsesocial.com/papers/6aa11d59cc3ad464a07d44cb https://doi.org/10.1039/c7ee01782k

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Synapse has enriched 5 closely related papers on similar clinical questions. Consider them for comparative context:

1Li2MnO3-stabilized LiMO2 (M = Mn, Ni, Co) electrodes for lithium-ion batteriesOriginal Research · 2007 · 2,039 citations
2Insight into the Atomic Structure of Cycled Lithium-Rich Layered Oxide Li<sub>1.20</sub>Mn<sub>0.54</sub>Co<sub>0.13</sub>Ni<sub>0.13</sub>O<sub>2</sub> Using HAADF STEM and Electron NanodiffractionOriginal Research · 2014 · 151 citations
3Electrochemical Activities in Li[sub 2]MnO[sub 3]Original Research · 2009 · 383 citations
4The Effects of Acid Treatment on the Electrochemical Properties of 0.5 Li[sub 2]MnO[sub 3]⋅0.5 LiNi[sub 0.44]Co[sub 0.25]Mn[sub 0.31]O[sub 2] Electrodes in Lithium CellsOriginal Research · 2006 · 276 citations
5Structural evolution and the capacity fade mechanism upon long-term cycling in Li-rich cathode materialOriginal Research · 2012 · 223 citations

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First-charge instabilities of layered-layered lithium-ion-battery materials2015
Review of the U.S. Department of Energy’s “Deep Dive” Effort to Understand Voltage Fade in Li- and Mn-Rich Cathodes2015

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