Make intergrowth, not war! Hierarchically organized MFI zeolites with micro-, meso-, and macroporosity (see scheme) in one structure were made by sequential intergrowth by using a simple organic structure-directing agent (OSDA) without meso- or macroporogens. The use of an OSDA that imperfectly fits the zeolite framework generated very thin zeolite plates with 90° rotational intergrowth.
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Chaikittisilp et al. (2013) studied this question.
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