Crystals of (15-crown-5)2KTCNQ adopt a solid-state architecture built up from isolated TCNQ•- dimer units surrounded by crown-encapsulated cation “barrels” with no evidence for direct counterion interaction. The structural and spectroscopic behavior of this material therefore provides a valuable model for the solid-state behavior of an isolated TCNQ•- dimer.
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Grossel et al. (1996) studied this question.
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