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February 18, 2013Angewandte Chemie

Efficient Oxidation of Methane to Methanol by Dioxygen Mediated by Tricopper Clusters

Sunney I. Chan Yu‐Jhang Lu Penumaka Nagababu Suman Maji Mu‐Cheng Hung Marianne M. Lee I‐Jui Hsu Pham Dinh Minh Jeff C.‐H. Lai Kok Yoah Ng Sridevi Ramalingam Steve S.‐F. Yu Michael K. Chan

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Abstract

Zwei Trikupfer-Komplexe wurden entwickelt, die die effiziente Oxidation von Methan zu Methanol unter Umgebungsbedingungen vermitteln: ein biomimetischer Trikupfer-Komplex (siehe Bild) und eine von der Methan-Monooxygenase (pMMO) abgeleitete Trikupferpeptid-Spezies.

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Cite This Study

Chan et al. (2013) studied this question.

synapsesocial.com/papers/6aa375cf22af0bded4f42443 https://doi.org/10.1002/ange.201209846

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Synapse has enriched 5 closely related papers on similar clinical questions. Consider them for comparative context:

1Current challenges of modeling diiron enzyme active sites for dioxygen activation by biomimetic synthetic complexesReview · 2010 · 299 citations
2Controlled Oxidation of Hydrocarbons by the Membrane-Bound Methane Monooxygenase: The Case for a Tricopper ClusterOriginal Research · 2008 · 206 citations
3Efficient Room‐Temperature Oxidation of Hydrocarbons Mediated by Tricopper Cluster Complexes with Different LigandsOriginal Research · 2012 · 44 citations
4Facile O-atom insertion into CC and CH bonds by a trinuclear copper complex designed to harness a singlet oxeneOriginal Research · 2007 · 86 citations
5Dioxygen Activation of a Trinuclear Cu<sup>I</sup>Cu<sup>I</sup>Cu<sup>I</sup> Cluster Capable of Mediating Facile Oxidation of Organic Substrates: Competition between O‐Atom Transfer and Abortive Intercomplex ReductionOriginal Research · 2012 · 42 citations

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Redox Potentiometry Studies of Particulate Methane Monooxygenase: Support for a Trinuclear Copper Cluster Active Site2007
Redox Potentiometry Studies of Particulate Methane Monooxygenase: Support for a Trinuclear Copper Cluster Active Site2007
The Copper Clusters in the Particulate Methane Monooxygenase (pMMO) from Methylococcus Capsulatus (Bath)2004

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