Energy breakdown: Photodissociation of mercaptan in the second absorption band has been studied by velocity map imaging. CH3 fragment images (see figure) show a structure directly related to the vibrational population of the SH counterfragment. An inverted SH vibrational population has been measured suggesting a non-adiabatic fast photodissociation.
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Izquierdo et al. (2006) studied this question.
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