An experiment studying the influence of molecular rotation in HI on photoelectron-spin polarization is presented. The experiment is highly wavelength selective since a laser-based vacuum-ultraviolet-radiation source with a bandwidth of 0.5×{}10^-4 nm is applied to produce circularly polarized light. Although in the Fano effect the kinetic energy of the photoelectrons is not analyzed, rotational structure is resolved via narrow-band excitation of autoionization resonances. The photoelectron-spin polarization is found to be strongly affected by the rotational substructure, leading to changes in both magnitude and sign for different rotational lines.
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Huth‐Fehre et al. (1990) studied this question.
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