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January 1, 2019Catalysis Science & Technology

Active sites and mechanism of the direct conversion of methane and carbon dioxide to acetic acid over the zinc-modified H-ZSM-5 zeolite

Peng Zhang Xuejing Yang Xiuli Hou Jianli Mi Zhizhong Yuan Jun Huang Catherine Stampfl

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Abstract

The catalytic activity of the conversion of CH 4 and CO 2 on zinc modified H-ZSM-5 is strongly dependent on the structure of the active sites.

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Zhang et al. (2019) studied this question.

synapsesocial.com/papers/6aa7cd0c5a44c3b67fae5b06 https://doi.org/10.1039/c9cy01749f

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Synapse has enriched 5 closely related papers on similar clinical questions. Consider them for comparative context:

1Direct C–C Coupling of CO<sub>2</sub> and the Methyl Group from CH<sub>4</sub> Activation through Facile Insertion of CO<sub>2</sub> into Zn–CH<sub>3</sub> σ-BondOriginal Research · 2016 · 134 citations
2Mechanistic Insight into the Formation of Acetic Acid from the Direct Conversion of Methane and Carbon Dioxide on Zinc-Modified H–ZSM-5 ZeoliteOriginal Research · 2013 · 193 citations
3Density Functional Theory (DFT) Study To Unravel the Catalytic Properties of M-Exchanged MFI, (M = Be, Co, Cu, Mg, Mn, Zn) for the Conversion of Methane and Carbon Dioxide to Acetic AcidOriginal Research · 2017 · 93 citations
4Active Site Ensembles Enabled C–C Coupling of CO<sub>2</sub> and CH<sub>4</sub> for Acetone ProductionOriginal Research · 2018 · 19 citations
5First-Principles Kinetic Study on the Effect of the Zeolite Framework on 1-Butanol DehydrationOriginal Research · 2016 · 57 citations

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Theoretical Insights into the Selective Oxidation of Methane to Methanol in Copper-Exchanged Mordenite2016
Monocopper Active Site for Partial Methane Oxidation in Cu-Exchanged 8MR Zeolites2016
Methane to Acetic Acid over Cu-Exchanged Zeolites: Mechanistic Insights from a Site-Specific Carbonylation Reaction2015

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