If the hat fits: The size of the ferrocene coligands used during the self-asssembly of hexaazatriphenylene hexacarbonitrile (hat-(CN)6) with CuI ions determines the coordination mode of the hat-(CN)6 ligand (bipyridine chelation or monodentate CN, see picture). The mode of coordination directly affects the oxidation state and the reduction potentials of the hat-(CN)6 ligand.
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Furukawa et al. (2005) studied this question.
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