Generalized Model for Photoinduced Surface Structure in Amorphous Thin Films

We present a generalized model to explain the spatial and temporal evolution of photoinduced surface structure in photosensitive amorphous thin films. The model describes these films as an incompressible viscous fluid driven by a photoinduced pressure originating from dipole rearrangement. This derivation requires only the polarizability, viscosity and surface tension of the system. Using values of these physical parameters, we check the validity of the model by fitting to experimental data of As2S3 and demonstrating good agreement.