Fits to spectral energy levels for Ho3+:LaCl3 and Gd3+:LaCl3 establish, for the first time, empirical values of the lanthanide spin-correlated crystal field parameters. The fitted rank 6 parameters are consistent with the superposition model analysis and provide the solution to a long standing problem in the fitted values of the crystal field parameters for trivalent lanthanide ions in LaCl3.
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Crosswhite et al. (1984) studied this question.
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