The expression for driving force is presented for multicomponent gas hydrate nucleation in an aqueous phase. The derivation includes working equations for predicting the composition of a hydrate nucleus. The results for driving force in multicomponent systems show a significant effect of the composition of the hydrate nucleus. All past work assume a fixed composition based on the three-phase equilibrium point independent of subcooling and supersaturation.
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Anklam et al. (2004) studied this question.
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