A one‐dimensional (1D) arrangement of an unsubstituted partially oxidized Dy3+ double‐decker complex, [DyPc2]Ix (Pc=phthalocyaninato, I=iodide; 1.93 1), was obtained by using electro‐oxidation and chemical oxidation. In 1, the Pc ligands were partially oxidized, and I3− ion was present as a counter ion. From the results of spectrophotometric analysis on 1, the π radicals were delocalized in a 1D column and behaved as a conductor even at low‐temperatures. Since conductivity was observed at temperatures lower than the blocking temperature (TB), magnetoresistance (MR) effects corresponding to a magnetic hysteresis of single‐molecule magnet (SMM) were observed when the galvanomagnetic characteristics were investigated at 2.2 K.
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Sato et al. (2021) studied this question.
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