Measurements of viscosity, ultrasonic velocity, refractive index, and density of chitosan (CS)/polyethylene glycol (PEG) blends in buffer solution (0.1 M acetic acid+0.2 M sodium acetate) were carried out for different blend compositions at 30, 40, and 50°C. Using the viscosity data, interaction parameters μ and α were computed to determine miscibility. These values revealed that the blend was miscible when the chitosan content was more than 60% of the blend. The results were further confirmed by ultrasonic velocity, density, and refractive index measurements. Further, the results revealed that the change in temperature has no significant effect on the miscibility of CS/PEG polymer blends.
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Jayaraju et al. (2006) studied this question.