All-Perovskite Photodetector with Fast Response

Perovskites have attracted substantial attention on account of their excellent physical properties and simple preparation process. Here we demonstrated an improved photodetector based on solution-processing organic-inorganic hybrid perovskite CH 3 NH 3 PbI 3− x Cl x layer decorated with CsPbBr 3 perovskite quantum dots. The CH 3 NH 3 PbI 3− x Cl x -CsPbBr 3 photodetector was operated in a visible light region, which appeared high responsivity ( R = 0.39 A/W), detectivity ( D* = 5.43 × 10 9 Jones), carrier mobility ( μ p = 172 cm 2 V −1 s −1 and μ n = 216 cm 2 V −1 s −1 ), and fast response (rise time 121 μs and fall time 107 μs). The CH 3 NH 3 PbI 3− x Cl x -CsPbBr 3 heterostructure is anticipated to find comprehensive applications in future high-performance photoelectronic devices.