We report a two-color frequency domain triply vibrationally enhanced (TRIVE) four-wave mixing (FWM) method that is fully resonant and provides coherent multidimensional vibrational spectra. Temporal and spectral discrimination allow control of the coherent interference of multiple pathways including isolation of a specific pathway and coherent control of the relative intensities of peaks in a 2D spectrum. The method is the coherent analogue to two-color pump−probe spectroscopy and allows the dissection of the individual pathways.
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Meyer et al. (2004) studied this question.
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