The NO2 radical was studied by E.S.R. in X-irradiated single crystals of NaNO3. At room temperature the spectrum was interpreted as due to NO2 rotating about the C 3 axis of the parent NO3 - ion. At 77K the motion is frozen and the radical is trapped at three distinct sites in the crystal. 14N and 17O hyperfine tensors for both rotating and static NO2 were measured
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Silver et al. (1971) studied this question.
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