The isosteric heat of adsorption of methane in an activated carbon adsorbent has been modeled by Monte Carlo simulation, using a pore-size distribution (PSD) to relate simulation results for pores of different sizes to the experimental adsorbent. Excellent fits were obtained between experimental and simulated isosteric heats of adsorption of methane in BPL activated carbon. The PSD was then used to predict the adsorption of methane and ethane in the same carbon adsorbent, with good results. The PSD derived from isosteric heat data was shown to be richer in information than PSDs obtained by the more conventional method of fitting to isotherm data.
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He et al. (2005) studied this question.
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