A time-dependent quantum theory of multiphoton ionization and dissociation is presented. The novel and crucial feature is the use of Floquet amplitudes from semiclassical radiation theory in an R-matrix theory based upon molecular R-matrix states dressed by photon number states. A simple numerical example is presented (time dependence of the one-photon dissociation yield from a square well).
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Leforestier et al. (1982) studied this question.
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