The potential-controlled electron-transfer reaction between cytochrome c and 1,1‘-dimethylferrocene at a liquid−liquid interface is reported. In this new approach to protein electrochemistry, the electron transfer process is apparently transport controlled, rather than adsorption limited. Furthermore, electron transfer at the liquid−liquid interface more closely resembles the situation of the protein in vivo.
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Lillie et al. (2002) studied this question.
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