We extend our generalized Langevin equation for cooperative dynamics (CDGLE), a many-chain approach, to investigate liquids composed of macromolecules with different local chemical structure. In particular, the specific role of semiflexibility and local architecture on the overall polymer dynamics is explored. The theory predicts centre-of-mass diffusion in good agreement with simulations for liquids of macromolecules with slightly branched monomeric architectures.
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Sambriski et al. (2007) studied this question.
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