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A density functional pseudopotential formalism is used to calculate the heat of formation and the volume of formation of disordered solid alloys formed by two alkali metals and two alkali-earth metals. The results are then analysed in terms of the semi-empirical parameters (electronegativity, charge transfer and interstitial electron density) often used in the semi-empirical descriptions of the alloy formation process.
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Iñiguez et al. (1982) studied this question.
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