Fourier path integral Monte Carlo simulations are used to demonstrate that in isotopically mixed clusters mass differences can lead to a purely quantum analog of classical binary phase separation. A parametric multistage sampling method is developed to simulate such systems, and results are presented for the strongly quantum mechanical p-H₂/o-D₂ and the quasiclassical ²⁰Ne/²²Ne binary clusters.
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Charusita Chakravarty (1995) studied this question.
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