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July 5, 2024Organic Letters16 citations

Palladium-Catalyzed Asymmetric Desymmetrization for the Simultaneous Construction of Chiral Phosphorus and Quaternary Carbon Stereocenters

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HZHengrui ZhouYXYiji XueXZXiang Zhou

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Abstract

A palladium-catalyzed asymmetric tandem Heck and carbonylation of bisallyl-phosphine oxides has been developed. This desymmetrization process provided an efficient route to the simultaneous synthesis of a chiral P-stereogenic center and a chiral quaternary carbon stereocenter in good yields with good diastereo- and enantioselectivities.

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Zhou et al. (2024) studied this question.

synapsesocial.com/papers/68e613bcb6db6435875a6405https://doi.org/10.1021/acs.orglett.4c01863
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