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February 28, 20260 citationsOpen Access

Atomic-Scale Optical Microscopy with Continuous-Wave Mid-Infrared Radiation

FSFelix SchieglVBValentin BergbauerSNSvenja Nerreter

Key Points

  • The aim is to achieve atomic-scale optical microscopy through enhanced spatial resolution using continuous-wave mid-infrared radiation.
  • Utilized a tabletop continuous-wave mid-infrared laser for optical microscopy
  • Employed intensity-based detection to observe optical signals
  • Analyzed the impact of anharmonic tip oscillation on optical signals
  • Achieved optical signals modulated on Ångstrom length scales
  • Identified tunneling currents as the source of emitted light
  • Proposed strategies to mitigate detrimental anharmonic oscillation effects

Abstract

Understanding matter at the most fundamental level requires optical microscopy with ever-higher spatial resolution. Scanning near-field optical microscopy (SNOM) has enabled important advances, circumventing the diffraction limit of light by confining it to the apex of a sharp metallic tip. However, the mesoscopic tip geometry restricts the spatial resolution to the nanometer scale. Here, using a conventional tabletop continuous-wave mid-infrared laser and intensity-based detection we observe optical signals modulated on Ångstrom length scales, consistent with light emission from atomically confined tunneling currents. The emergence of near-field optical tunneling emission (NOTE) ─ considered a strong-field excitation process ─ under continuous-wave driving is remarkable, as it typically requires ultrashort high-intensity laser pulses. Further, we find that anharmonic tip oscillation can influence the signal and propose strategies to mitigate this effect. Our findings enable the use of this tunneling-mediated contrast mechanism with standard optical setups, establishing a pathway to optical imaging with unprecedented resolution.

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Cite This Study

Schiegl et al. (2026) studied this question.

synapsesocial.com/papers/69a286240a974eb0d3c00d93https://doi.org/10.5283/epub.78709
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