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March 7, 2026Analytical Chemistry1 citations

Nested Ring Resonant Sagnac-Enhanced Photothermal Gas Sensing Using a Nanofiber

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FWFu WanLZLei ZhuYBYaotian Bai

Key Points

  • This research aims to develop a highly sensitive photothermal gas sensor using a novel nested ring resonant Sagnac design.
  • Developed a nested ring resonator within a Sagnac loop using a 2 cm-long nanofiber.
  • Measured sensitivity through the noise equivalent concentration of C2H2 detection.
  • Compared performance with a nonresonant Sagnac interferometer using the same nanofiber.
  • Achieved a noise equivalent concentration of 16 ppb for C2H2 detection.
  • Demonstrated a response time of 19 seconds and less than 3% instability over 2 hours.
  • Improved sensitivity by a factor of 10 compared to the nonresonant Sagnac configuration.

Abstract

Photothermal (PT) spectroscopy exhibits exceptional selectivity and high sensitivity for trace gas detection, yet developing PT gas sensors that combine fast response, high sensitivity, and practical usability remains a significant challenge. Here, we demonstrate a nested ring resonant Sagnac-enhanced PT gas sensor using a nanofiber. By inserting a nested ring resonator within the Sagnac loop, the proposed sensor reduces the full width at half-maximum of the resonance peak, thereby enhancing the cavity finesse and improving the sensitivity of PT phase modulation. With a 2 cm-long nanofiber and a resonator finesse of 73, the sensor achieves precise C2H2 detection featuring a noise equivalent concentration of 16 ppb, a 19 s response time, and <3% instability over 2 h. Compared to a nonresonant Sagnac interferometer using the same nanofiber, this configuration improves sensitivity by a factor of 10. By amplifying the PT effect within a short nanofiber, the sensor successfully integrates fast response with high sensitivity, overcoming the response delay typically associated with long sensing fibers. Furthermore, the sensor operates without complex wavelength-locking mechanisms, simplifying its operation and rendering it suitable for applications in remote monitoring and distributed sensing networks.

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Cite This Study

Wan et al. (2026) studied this question.

synapsesocial.com/papers/69abc1955af8044f7a4ea608https://doi.org/10.1021/acs.analchem.5c05900
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