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August 14, 2025

Synergistic Multi-Field Regulation via MOF-Polymer Hybrid Separators Enabling Dendrite-Free and Thermally Stable Lithium Metal Batteries.

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Authors

FXFan XuUniversity of Shanghai for Science and TechnologyLZLanlan ZuoNational University of Defense TechnologyXSXianxian ShiNational University of Defense Technology

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Overview

Composite separator demonstrates improved thermal stability and suppresses dendrite growth in lithium metal batteries, indicating enhanced performance.

Key Points

  • The multifunctional separator significantly reduces dendrite growth in lithium metal batteries.
  • It achieves a high Li+ transference number of 0.96 through innovative ion transport regulation.
  • The NCM811||Li cells retain 89.3% capacity after 200 cycles, showcasing durability in performance.
  • Superior thermal regulation allows the separator to maintain structural integrity at extreme temperatures up to 150 °C.

Cite This Study

Xu et al. (2025) studied this question.

synapsesocial.com/papers/689fc6912abb084d53ed266fhttps://doi.org/10.1021/acsnano.5c06984
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Also Consider

Synapse has enriched 5 closely related papers on similar clinical questions. Consider them for comparative context:

  1. 1Dual-functional Separators Regulating Ion Transport Enabled by 3D-Reinforced Polyimide Microspheres Protective Layer for Dendrite-Free and High-Temperature Lithium Metal Batteries2024 · 6 citations
  2. 2A Porous Polyimide Composite Separator with an In Situ-Polymerized PDOL Gel Network for Enhanced Dendrite Suppression and Interfacial Stability in Lithium-Metal Batteries2026 · 1 citations
  3. 3Permselective Metal–Organic Framework-Based Separators via In Situ Self-Assembly for High-Performance Lithium Metal Batteries2024 · 12 citations
  4. 4Mixed-Linker Metal–Organic Frameworks Modified Separators as Li+-Transport Accelerators for Wide-Temperature and Long-Cycling Lithium Metal Batteries2026
  5. 5Janus Bilayer Separator With Opposite Charges for Lithium Metal Batteries2026