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August 11, 2025

Modeling Single-Crystal Electrodes as a Network of Primary Particles

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Authors

POPierfrancesco OmbriniSPShakul PathakDNDimitrios Ntagkras

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Overview

Modeling predicts voltage response of LiFePO4 electrodes, suggesting enhanced charge transport in single-crystal systems.

Key Points

  • The model predicts voltage responses of LiFePO4 electrodes without empirical tuning, demonstrating robust performance across varied conditions.
  • Voltage response and charge-discharge behavior are accurately captured, highlighting significant asymmetries and hysteresis.
  • This approach utilizes a physics-based framework, linking particle-scale interactions to overall cell performance effectively.
  • The study proposes a computationally efficient model for single-crystal electrodes, supporting future designs and control through validated kinetics.

Cite This Study

Ombrini et al. (2025) studied this question.

synapsesocial.com/papers/68a35ef30a429f79733283dahttps://doi.org/10.26434/chemrxiv-2025-80lsd
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