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August 19, 2025Nature CommunicationsOpen Access

Pd nanocatalysts engineering for direct oxidation methane-to-methanol with 99.7% selectivity

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Authors

PDPeilin DengYXYueshan XuDWDaoxiong Wu

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Overview

Experiment shows Pd crystal facet type affects methane-to-methanol conversion, highlighting structure-performance links in catalysts.

Key Points

  • Exceptional CH3OH yield of 201.8 mmol·gPd−1·h−1 achieved using {111}-faceted Pd nanocrystals.
  • Pd {111} facet weakens adsorption strength of intermediates, promoting H2O2 and CH3OH production.
  • Synthesis of well-defined Pd nanocrystals enables investigation of structural effects on performance.
  • Insights gained may guide the design of efficient catalysts for methane-to-methanol conversion.

Cite This Study

Deng et al. (2025) studied this question.

synapsesocial.com/papers/68af474ead7bf08b1ead3ac2https://doi.org/10.1038/s41467-025-63067-0
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Also Consider

Synapse has enriched 5 closely related papers on similar clinical questions. Consider them for comparative context:

  1. 1Operando TEM Study of Partial Oxidation of Methane Over Pd Nanoparticles2025 · 3 citations
  2. 2Three-Dimensionally Ordered Macroporous Superstructure of Nitrogen-Doped Hierarchical Porous Carbon Implanted with Ultrafine Pd Nanoclusters for the Efficient Methanol Oxidation Reaction2026
  3. 3Precisely Modulating the Interfacial Oxygen Radicals for Selective Photocatalytic Methane Partial Oxidation to Methanol2026
  4. 4Precisely Modulating the Interfacial Oxygen Radicals for Selective Photocatalytic Methane Partial Oxidation to Methanol2026
  5. 5Operando Investigations of Structure-Activity Relationships in Pd-based Model Catalysts for Methane Oxidation2026