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September 5, 2025Science Advances

Capturing carbon monoxide—Accessing bis(boryl)ketones through direct B–B bond carbonylation

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Carbon monoxide directly engages B-B bonds from tetraborane, leading to new boryl ketones, highlighting their unique properties.

Carbon monoxide significantly modifies B-B bonds to create rare boryl ketones, expanding their synthetic potential.
The study reports stable carbonyl compounds, with one showing impressive thermal stability while another is thermally rearranged.
Boron heterocycles exhibit interesting reduction processes, producing radical monoanion and dianion species while maintaining structure.
Analytical and theoretical methods reveal unique characteristics of these boron-carbonyl compounds, underscoring their synthetic utility.

Beck et al. (2025) studied this question.

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