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Resonant x-ray spectroscopies on CrSBr: Probing the electronic structure through chromium d−d excitations

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Significant linear dichroism in CrSBr highlights its unusual electronic structure and excitonic behavior, which can inform future applications.
Excitations were investigated through resonant inelastic x-ray scattering and x-ray absorption spectroscopy, providing essential insights into the material’s properties.
A multiplet model based on crystal field theory was developed, successfully explaining several observed features while revealing hybridization complexities.
These findings not only enhance our knowledge of the electronic structure in CrSBr, but also serve as groundwork for further studies in spintronic applications.

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Analysis of electronic excitations in CrSBr reveals linear dichroism and d-d transitions, indicating novel excitonic properties.

Porée et al. (2025) studied this question.

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