Plasma-derived hydrogen radical-mediated N2 activation for mild ammonia synthesis: insights into the importance of the oxygen vacancy on the reaction mechanism

Shijian Luo; Yongduo Liu; Lin Guo; Yang Song; Yuran Yang; Fadong Chen; L Wang; Yanan Chen; Siguo Chen; Zidong Wei

doi:10.1039/d5ta04447b

January 1, 2025Journal of Materials Chemistry A

Plasma-derived hydrogen radical-mediated N2 activation for mild ammonia synthesis: insights into the importance of the oxygen vacancy on the reaction mechanism

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Key Points

Efficient N2 activation reduces barriers for ammonia synthesis, enabling decentralized production.
This method improves ammonia yields compared to traditional processes, emphasizing the reaction mechanism's role.
Assessment using plasma-catalytic techniques reveals the importance of oxygen vacancy in the synthesis process.
These findings support advancements in sustainable nitrogen fixation technologies for improved ammonia synthesis.

Implication

This study demonstrates efficient N2 activation for NH3 production, highlighting the role of oxygen vacancy.

Abstract

Plasma-catalytic NH3 synthesis has recently been recognized as a complementary route to the Haber–Bosch process for decentralized NH3 production. However, the activation of N2 in current plasma catalysis works is...

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Cite This Study

Luo et al. (2025) studied this question.

synapsesocial.com/papers/68c19f9154b1d3bfb60dae64 https://doi.org/10.1039/d5ta04447b

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Plasma-derived hydrogen radical-mediated N2 activation for mild ammonia synthesis: insights into the importance of the oxygen vacancy on the reaction mechanism

Key Points

Implication

Abstract

Discussion

Cite This Study

Plasma-derived hydrogen radical-mediated N2 activation for mild ammonia synthesis: insights into the importance of the oxygen vacancy on the reaction mechanism

Key Points

Implication

Abstract

Discussion

Cite This Study

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