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Aminoalkylation of Alkenes for Modular Pyrrolidine Synthesis via Electron Donor–Acceptor Complexes Generated from Alkenes and Amine-Tethered N-Hydroxyphthalimide Esters

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Catalyst-free aminoalkylation shows broad substrate scope in alkenes and NHPI esters, suggesting modular synthesis.

This method enables rapid synthesis of various nitrogen-containing heterocycles, improving accessibility.
EDA complex formation facilitates the reaction, which produces a broad array of products efficiently.
Visible-light induction eliminates the need for external catalysts, making the process simpler and more sustainable.
The versatility in substrate choice suggests potential applications in biologically relevant compound synthesis.

Tayu et al. (2025) studied this question.

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