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September 14, 2025

A Hybrid Ultrastrong Coordinating Solvent and an Ion-Conductive Diluent for High-Voltage Ether-Based Li-Metal Batteries.

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Authors

XXXiaoxin XieJFJuanjuan FuRWRuoxi Wang

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Overview

This research shows improved electrochemical performance in Li-metal batteries, highlighting the role of ether coordination and interfacial stability.

Key Points

  • The hybrid electrolyte utilizing 12-crown-4 showed significant improvement in ionic conductivity and cycling stability.
  • Weak coordinating ethers enable faster Li+ desolvation, enhancing performance with the Li-metal anode.
  • Interfacial passivators like lithium bis(fluorosulfonyl)imide further elevate cell performance.
  • This study proposes a new electrolyte design paradigm for high-voltage ether electrolytes.

Cite This Study

Xie et al. (2025) studied this question.

synapsesocial.com/papers/68c6df6933b72be0b5e43cachttps://doi.org/10.1021/jacs.5c07899
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