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Photodissociation Dynamics in (N₂)n⁺ Clusters

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Photodissociation of N2 clusters reveals complex dynamics, particularly for larger clusters where N4+ plays a crucial role.
During UV laser exposure, all cluster sizes absorb strongly around 355 nm, leading to the release of N2+ and N4+ fragments.
Kinetic energy release analysis demonstrates significant energy values during dissociation, indicating N4+ ions are near the surface of clusters.
Larger N2 clusters dissociate with consistent energy values, suggesting limited influence from clustering on the N2+ and N4+ kinetic energy.

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Velocity-map imaging uncovers photodissociation dynamics in N2 clusters, highlighting N4+ as a key chromophore.

Blais et al. (2025) studied this question.

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