Scanning tunneling microscopy reveals molecular switch chain assembly on lead at 0.3 K, indicating substrate faceting and persistent spin-flip excitations.
A complex based on a Ni(II) porphyrin exhibiting spin crossover on Ag(111) is studied on Pb(100) by scanning tunneling microscopy at 0.3 K. Strong molecular interactions between the phenyl and pentafluorophenyl moieties lead to the formation of molecular chains and cause a faceting of the substrate surface. The chains are located along double and multiple substrate steps that deviate from high-symmetry directions. Tunneling spectroscopy reveals spin-flip excitations of an
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Treichel et al. (2024) studied this question.
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