Z₂ flux binding to higher-spin impurities in the Kitaev spin liquid: mechanisms and implications

Stabilizing Z₂ fluxes in Kitaev spin liquids (KSLs) is crucial for both characterizing candidate materials and identifying Ising anyons. In this study, we investigate the effects of spin-S magnetic impurities embedded in the spin-1/2 KSL. Utilizing exact diagonalization and density matrix renormalization group methods, we examine the impurity magnetization and ground-state flux sector with varying impurity coupling and spin size. Our findings reveal that impurity magnetization exhibits an integer/half-integer spin dependence, which aligns with analytical predictions, and a flux-sector transition from bound-flux to zero-flux occurs at low coupling strengths, independent of the impurity spin. Notably, for spin-3/2 impurities, we observe a reentrant bound-flux sector, which remains stable under magnetic fields. By introducing a minimal model based on Majorana fermions, we provide phenomenological explanations for the transitions. Our results suggest a novel way of binding a flux in KSLs, beyond the proposals of vacancies or Kondo impurities.