Experimental study reveals a spectral gap without magnetic ordering in triangular lattice NaYbSe2, suggesting a gapped Z2 quantum spin liquid.
We report neutron scattering, pressure-dependent AC calorimetry, and AC magnetic susceptibility measurements of triangular lattice NaYbSe₂. We observe a continuum of scattering, which is reproduced by matrix product simulations, and no phase transition is detected in any bulk measurements. Comparison to heat capacity simulations suggest the material is within the Heisenberg spin liquid phase. AC Susceptibility shows a significant 23~mK downturn, indicating a gap in the magnetic spectrum. The combination of a gap with no detectable magnetic order, comparison to theoretical models, and comparison to other AYbSe₂ compounds all strongly indicate NaYbSe₂ is within the quantum spin liquid phase. The gap also allows us to rule out a gapless Dirac spin liquid, with a gapped Z₂ liquid the most natural explanation.
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Scheie et al. (2024) studied this question.
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