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October 8, 2025ACS Applied Materials & Interfaces

Submicrometer Lithiophilic Interphase Layer Engineering toward Inorganic-Rich Solid Electrolyte Interphase for High-Performance Anode-Free Lithium Metal Batteries

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Authors

XFXiaoming FanZSZhiwei ShiTZTao Zuo

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Overview

This research demonstrates enhanced cycling stability and Coulombic efficiency in anode-free lithium metal batteries with improved lithiophilic interphase layers.

Key Points

  • Achieving a Coulombic efficiency of 98.5% over 650 cycles highlights the effectiveness of the lithiophilic interphase layer in battery performance.
  • The introduction of silver nanoparticles enhances Li+ transportation and the lithiophilic feature of the copper substrate, improving lithium deposition.
  • Development of a submicrometer interphase layer based on silica nanospheres promotes the formation of a robust solid electrolyte interphase rich in inorganic compounds.
  • This approach offers a scalable method for engineering high-performance anode-free lithium metal batteries while minimizing energy density loss.

Cite This Study

Fan et al. (2025) studied this question.

synapsesocial.com/papers/68e6679587ecc93a24d17480https://doi.org/10.1021/acsami.5c12477
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