Dual grating single-shot pump-probe technique

A simple and effective single-shot pump-probe technique is reported. Using only two commercial gratings, a large time window of 95.4 ps is spatially encoded in a single probe pulse, and single-shot time-resolved measurements are implemented. The time window exceeds the maximum reported values for single-shot pump-probe techniques using the echelon or angle beam encoding strategy. The phase difference problem in the echelon encoding strategies is also eliminated and a customized echelon is not needed in this technique. The measurements of the ultrafast two-photon absorption dynamics of ZnSe at a wavelength of 650 nm verify the effectiveness of this technique.