We present measurements of the electronic absorption spectrum of He-tagged buckminsterfullerene anions, <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:mrow><a:msub><a:mi mathvariant="normal">C</a:mi><a:mn>60</a:mn></a:msub><a:msup><a:mrow/><a:mo>−</a:mo></a:msup></a:mrow></a:math>. Using a technique that allows for the efficient tagging of complex molecular anions with He, we achieve atomically resolved action spectra that provide an accurate determination of the gas-phase absorption spectrum in the near-infrared regime. In total we identify 27 absorption bands between 895 and 1057 nm. Published by the American Physical Society 2024
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