Continuum of spin excitations observed in inelastic neutron scattering experiments are often considered as a strong evidence of quantum spin liquid formation. When quantum spin liquid is indeed the ground state of a disorder-free magnetic compound, the elementary excitation is no longer the conventional spin waves (magnons). Instead, the magnons fractionalize into spinons, leaving only a two-spinon continuum detectable in inelastic neutron scattering experiments. For a clean ordered antiferromagnet, it was unclear if we can observe a continuous spectrum similar to the ones in a quantum spin liquid state. Here we show that the magnetically ordered state in Na₂BaCo(PO₄)₂ is able to host a spin excitation continuum induced by strong quantum fluctuations. Thus, a second thought is necessary when concluding such continuum as signature of quantum spin liquid in new material explorations.
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Sheng et al. (2024) studied this question.
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