Implementation and Applications of a Precision Weak-Field Sample Environment for Polarized Neutron Reflectometry at J-PARC

Polarized neutron reflectometry (PNR) analyzes surface and interfacial structures of materials. For the SHARAKU reflectometer at the Materials and Life Science Experimental Facility in the Japan Proton Accelerator Research Complex, precise measurements under weak magnetic fields, which are critical for modern spintronics, have long been challenging. To address this issue, we developed a precise weak-field sample environment equipped with a newly designed coil system. The magnetic field at the sample position can be applied within the surface/interface plane, either in the scattering plane (horizontal configuration) or perpendicular to it (vertical configuration). The horizontal configuration achieved high polarization efficiency across a stable field range, whereas the vertical configuration enabled the experiments to cross zero into negative fields. We demonstrated the instrument’s capability by resolving the remanent magnetic structure of an Fe film. Its applicability to soft matter was proven through analysis of a cellulose thin film with roughness using magnetic contrast variation PNR. In this case, precise weak-field control is essential to tune the magnetic contrast from the reference layer beneath the soft film. These results establish the system as a versatile platform for future PNR and polarized off-specular scattering experiments across a wide range of materials.