This research analyzes spin-lattice relaxation times in metal-organic frameworks, suggesting differences from molecular crystals.
To rationalize the difference in spin–lattice relaxation times ( T 1 ) between metal–organic frameworks (MOF) and molecular crystals, their phonons and spin-phonon coupling were analysed using periodic density functional theory and Raman spectroscopy.
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Suzuki et al. (2026) studied this question.
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