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January 24, 2026ACS Applied Materials & Interfaces0 citationsOpen Access

Bio-Inspired Spike-Timing-Dependent Plasticity Learning with Metal Halide Perovskites: Toward Artificial Synaptic Functionality

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MSMostafa ShooshtariInstituto de Microelectrónica de SevillaSKSo-Yeon KimConsejo Superior de Investigaciones CientíficasSPSaeideh PahlavanInstituto de Microelectrónica de Sevilla

Key Points

  • The research aims to explore how halide perovskite memristors can simulate biological learning mechanisms like spike-timing-dependent plasticity.
  • Fabricated halide perovskite memristors (Cs3Bi2I6Br3) to study their behavior.
  • Developed a dynamic physical model to analyze voltage and history-dependent switching.
  • Utilized biphasic voltage pulses to replicate STDP characteristics during testing.
  • The memristor successfully mimicked classic STDP dynamics including long-term potentiation and long-term depression.
  • Maintained stable STDP behavior over 100 trials with less than 0.03% variation in synaptic weight.
  • Showcased advanced features like triplet-STDP and synaptic memory consolidation.

Abstract

Recent advances in neuromorphic engineering have sparked a convergence between nanotechnology and neuroscience, where emerging devices such as memristors are being explored to replicate fundamental learning mechanisms observed in the brain. One such mechanism, spike-timing-dependent plasticity (STDP), encodes synaptic changes based on the precise timing between pre- and postsynaptic spikes, and has been widely adopted in machine intelligence and computational neuroscience. In this work, we demonstrate that a halide perovskite memristor (Cs3Bi2I6Br3) can effectively simulate biologically plausible STDP dynamics. We fabricate and characterize the MHP-based device, and develop a dynamic physical model capturing its voltage- and history-dependent switching behavior. Using biologically inspired biphasic voltage pulses, the model replicates classic STDP characteristics including long-term potentiation (LTP), long-term depression (LTD), and the canonical asymmetric learning window. Further analysis shows that the memristor supports advanced features such as triplet-STDP and synaptic memory consolidation. Importantly, the STDP behavior remains stable across 100 independent trials with biologically realistic voltage noise, exhibiting less than 0.03% variation in synaptic weight. These results suggest that the inherent physical dynamics of halide perovskites enable bioinspired learning without external programming or algorithmic supervision. By bridging molecular-scale materials physics with spike-based computation, our findings lay the groundwork for implementing scalable, low-power, and noise-tolerant synaptic learning in next-generation neuromorphic computing systems.

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Cite This Study

Shooshtari et al. (2026) studied this question.

synapsesocial.com/papers/69746149bb9d90c67120b281https://doi.org/10.1021/acsami.5c21545
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