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February 12, 2026Physics of Fluids6 citations

Gas–liquid–solid coordinated transport behavior and pore clogging mechanisms during CO2 + O2 in situ leaching of sandstone-type uranium deposits

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FWFutian WangQNQinghe NiuWWWei (Vivian) Wang

Key Points

  • This research aims to understand the mechanisms and principles behind pore clogging during CO2 + O2 in situ leaching of uranium deposits.
  • Utilized a coupled volume of fluid-computational fluid dynamics-discrete element method approach.
  • Investigated fluid migration patterns under various conditions.
  • Examined the effects of particle size, rate, and reservoir properties on clogging.
  • Pore throat distribution and particle interactions influence fluid flow, leading to solid clogging.
  • Gas bubbles become trapped, causing gas clogging due to surface tension.
  • Increased particle irregularity and reservoir heterogeneity intensify clogging.
  • Higher fluid injection rates can reduce sedimentation and help to unclog pores.
  • Particle retention follows a logistic trend with injection rates and an exponential trend with particle size.

Abstract

The CO2 + O2in situ leaching (ISL) of sandstone-type uranium deposits faces the significant challenge of reservoir clogging, which has become a critical bottleneck limiting uranium resource extraction. This study employs a coupled volume of fluid-computational fluid dynamics-discrete element method to investigate the synergistic migration processes of gas, liquid, and solid phases under the influence of multiple factors, aiming to elucidate the mechanisms and governing principles of pore clogging in uranium reservoirs. Results show that the spatial distribution of pore throats and particle interactions alter fluid migration patterns, increasing the uncertainty of fluid flow and leading to solid clogging. CO2 + O2 moves with the leaching solution, forming a turbulent gas–liquid interface; some bubbles become trapped in pore throats due to surface tension, causing gas clogging. Increases in particle injection rate, particle size, particle irregularity, and reservoir heterogeneity all exacerbate pore clogging. Conversely, a higher fluid injection rate can reduce particle sedimentation and reactivate retained particles, promoting pore unclogging. The proportion of residual particles follows a logistic function trend with increasing particle and fluid injection rates and an exponential trend with particle diameter. Particle irregularity and reservoir heterogeneity increase the proportion of residual particles by factors of 2.13 and 1.12, respectively. For clogged uranium deposits, it is recommended to first apply chemical methods to reduce soluble mineral particles, then increase the leaching solution injection rate to mobilize retained particles, and finally employ low-amplitude, high-frequency reservoir stimulation for further unclogging. These strategies can extend the ISL mining lifespan and improve uranium recovery.

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Cite This Study

Wang et al. (2026) studied this question.

synapsesocial.com/papers/698d6dc15be6419ac0d52dc6https://doi.org/10.1063/5.0315059
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