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The study aims to explore ways to adjust the electronic properties of redox-active metalloligands for enhanced reactivity at metal centers.

February 21, 2026Chemical ScienceOpen Access

Tuning Reactivity at Uranium through Heterometal Substitution in a Redox-active Thiomolybdate Metalloligand

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The study aims to explore ways to adjust the electronic properties of redox-active metalloligands for enhanced reactivity at metal centers.
Utilized thiomolybdate metalloligands as platforms for reactivity tuning.
Implemented heterometal substitution to modify electronic properties.
Conducted electron transfer measurements to assess reactivity changes.
Achieved significant reactivity variations at uranium centers through specific heterometal substitutions.
Demonstrated that altered electronic properties correlated with enhanced multielectron transformations.
Identified optimal metal combinations for effective electron reservoir behavior.

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Research demonstrates reactivity tuning at uranium using heterometal substitution, indicating potential for new metallic transformations.

Valerio et al. (2026) studied this question.

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