Single-shot optical precessional magnetization switching of Pt/Co/Pt ferromagnetic trilayers

Ultra-fast magnetization switching triggered by a single femtosecond laser pulse has gained significant attention over the last decade for its potential in low-power consumption, high-speed memory applications. However, this phenomenon has been primarily observed in Gd-based ferrimagnetic materials, which are unsuitable for storage due to their weak perpendicular magnetic anisotropy (PMA). In this work, we demonstrated that applying a single laser pulse and an in-plane magnetic field can facilitate magnetic switching in a Pt/Co/Pt ferromagnetic trilayers stack within a specific laser power window. To further understand this phenomenon, we introduce a Cu layer to accelerate the re-establishment time of the anisotropy field of Pt/Co/Pt trilayers, which leads to bullseye-patterned magnetic switching. We have mapped phase diagram for these phenomena, and through micromagnetic simulations, we have determined that these switchings are influenced by thermal anisotropy torque, which can be modulated through PMA. These findings indicate that single-shot optical precessional magnetization reversal is feasible in a broader range of materials, opening avenues for the development of optical-magnetic memory devices.