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February 28, 2026Transformative EnergyOpen Access

A multi-scale model for PEMFC performance degradation coupled with catalyst layer microstructure evolution

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Authors

ZWZhixin WuYMYutong MuGZGuobin Zhang

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Overview

Dual-scale modeling demonstrates performance degradation mechanisms in proton exchange membrane fuel cells, suggesting improvements for durability.

Key Points

  • This study aims to develop a model to understand the relationship between microstructure evolution and performance degradation in PEMFCs under dynamic conditions.
  • Developed a dual-scale coupled model integrating 1D and 3D performance metrics
  • Analyzed critical degradation processes including platinum oxidation and carbon corrosion
  • Studied effects of operating conditions on performance degradation
  • Optimal operating temperature identified as 80°C for balance between kinetics and stability
  • Elevated upper potential limit to 1.1 V increases platinum dissolution and accelerates performance decay
  • Low platinum loading heightens mass transport polarization, leading to greater performance losses at high current densities

Cite This Study

Wu et al. (2026) studied this question.

synapsesocial.com/papers/69a285da0a974eb0d3c00cfdhttps://doi.org/10.1016/j.tegy.2026.100003
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